How Did Materialism Contribute To Augustine's Conversion?

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What hindered Augustine's conversion was that he was disillusioned in his pursuit of hedonism, paganism, Manicheanism, worldly power and ambition. He entertained the notion that ultimate truth might be simply unknowable or unattainable. He became impressed with the philosophical skepticism that had become prominent in Plato’s old school, the Academy. It was at this point that a number of factors began to come together that would lead Augustine to reassess the religion of his youth.
Some of the factors that fostered Augustine's conversion are: his interaction with the philosophy of Neo-Platonism helped him realize that materialism doesn't account for the moral and spiritual realities of life. Neoplatonic philosophy taught that while evil is

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