Ultrafast Processes

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Ultrafast Processes

Ultrafast optical phenomena refer to dynamical processes that occur in various forms of matter on the time scale of picoseconds or femtosecond. These phenomena have been relegated to the optical domain primarily because only lasers have been fast enough to probe many of these processes. This field of ukrtiast optical phenomena continues to be a highly prolific field of fundamental and applied research. One of the prime driving forces for the continued growth is the seemingly unending appearance of new and exotic sources of ultra short pulses and the concomitant proliferation of commercially available sources. Today, one can literally buy the pro-verbial “black-box” with the attached label – “femtosecond pulses exit here.”Driven by unprecedented levels of coherence, bandwidth, spectral diversity, high power, and small size, ultra short pulses of light have been utilized in fundamental studies of disciplines as diverse as semiconductor physics, plasma physics, Light wave transmission systems, and biological systems. In 1987, the Bell Labs group headed by Shank and Fork generated 6 fs du-ration optical pulse by coupling 30 fs, 2 TW/cm2 pulses (TW=Terawatt=l 012Watts) from an amplified colliding pulse mode locked (CPM) dye laser into a1-cm single-mode optical fibre and prism-grating compressor. After a decade of intense activity, tis 6 fs world record was finally broken by Wiersma’s group in The Netherlands – 5 fs via the fibre-prism-grating compression of in-tense 13 fs pulses fi-om a cavity-dumped Kerr-lens mode locked (KLM) Ti: sapphire laser. Limitations on the simultaneous control of the intracavity bandwidth and dispersion of KLM Ti:sapphire lasers has thus fw prevented the generation of pulses shorter than 7.5 fs directly from the laser oscillator –despite the fact that one can generate enough bandwidth in this laser system to support a 4 fs pulse!

SOME EXAMPLES OF ULTRAFAST PROCESSES

VIBRATION OF SMALL MOLECULES

FRAGMENTATION OF MOLECULES

ATOM-ATOM COLLISION

SOME OF THE OTHER ULTRA FAST PROCESSES

PROBING OF ULTRAFAST PROCESSES

The processes that occur in picoseconds and femtosecond time domain are called as ultrafast processes. So in order to study the dynamics of these fast processes we have to have a probing system in the same time domain. Ultrafast femtosecond pulses are used for the direct observation in the time scale for monitoring the physical and biological systems.

Ultra short laser pulses are considered to be those whose pulse duration is less than a few picoseconds (10-12 s) long. Recent research has led to techniques such as Kerr-lens mode locking to enable pulse duration down to around 5 femtoseconds (10-15 s) and chirped pulse amplification giving pulses peak powers of several terawatts.

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